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I don’t know what chain reaction exactly they were thinking of, but from modern fusion research, I believe we can confidently say that the atmosphere would need to be interior-of-a-large-star-level dense, and even then I’m not sure you’d get nitrogen fusing with anything without a lot of hydrogen or helium around. Nitrogen-nitrogen fusion seems extremely implausible for sure
Thank you, the page you sourced references a 2024 paper inspired by the Oppenheimer movie that was super interesting to read